Increasing soil organic carbon (SOC) stocks is a promising way to mitigate the increase in atmospheric CO2 concentration. Based on a simple ratio between CO2 anthropogenic emissions and SOC stocks worldwide, it has been suggested that a 0.4% (4 per 1000) yearly increase in SOC stocks could compensate for current anthropogenic CO2 emissions. Here, we used a reverse RothC modelling approach to estimate the amount of C inputs to soils required to sustain current SOC stocks and to increase them by 4 parts per thousand per year over a period of 30 years. We assessed the feasibility of this aspirational target first by comparing the required C input with net primary productivity (NPP) flowing to the soil, and second by considering the SOC saturation concept. Calculations were performed for mainland France, at a 1 km grid cell resolution. Results showed that a 30%-40% increase in C inputs to soil would be needed to obtain a 4 parts per thousand increase per year over a 30-year period. 88.4% of cropland areas were considered unsaturated in terms of mineral-associated SOC, but characterized by a below target C balance, that is, less NPP available than required to reach the 4 parts per thousand aspirational target. Conversely, 90.4% of unimproved grasslands were characterized by an above target C balance, that is, enough NPP to reach the 4 parts per thousand objective, but 59.1% were also saturated. The situation of improved grasslands and forests was more evenly distributed among the four categories (saturated vs. unsaturated and above vs below target C balance). Future data from soil monitoring networks should enable to validate these results. Overall, our results suggest that, for mainland France, priorities should be (1) to increase NPP returns in cropland soils that are unsaturated and have a below target carbon balance and (2) to preserve SOC stocks in other land uses.